Notably steroids steroids, among all bases screened, cesium carbonate (CsCO) plays a crucial role and enables reversibility in the first step with subsequent structure locking by formation of a C=C double bond to maintain crystallinity, which is supported by density functional theory (DFT) calculation. We propose a quantifiable energy diagram of a “quasireversible reaction” which allows to identify further suitable CC bond formation reactions for 2D polymerizations. Moreover, we delineate the narrowing of the HOMOLUMO gap by expanding conjugation into two dimensions.
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